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The three fugitive siblings accused of crimes in Florida and Georgia were arrested Wednesday following a car crash in southern Colorado, state police said.

Ryan Dougherty, 21, Dylan Dougherty, 26 and their sister, Lee Grace Doughtery, 29, were taken into custody after a short pursuit on Interstate 25 near Walsenburg, roughly 50 miles north of the New Mexico state line, according to the Colorado State Patrol.

The three are accused of firing at least 20 shots at a Florida police officer after a high-speed chase, and then robbing a Georgia bank at gunpoint. They were considered heavily armed and dangerous.

Witnesses near Colorado City first spotted the trio in a white Subaru headed south. Police and the suspects eventually engaged in a high-speed chase that lasted 20 miles, until their vehicle rolled over, according to reports. One brother ran from the car, but was swiftly apprehended by a state trooper, state police said.

On Tuesday, the search shifted to Colorado, where police and FBI officials say they believe the trio made a purchase at an outdoors shop and could be headed to a campground or rural area to try to avoid capture.

The weeklong search for the three siblings accused of crimes in Florida and Georgia sparked the nation’s interest and grew comparisons to Bonnie and Clyde because of their good looks and bravado.

Last Tuesday, a Zephyrhills, Fla., police officer attempted to pull the trio over for speeding near the Florida-Georgia border.

After the officer began chasing the vehicle, one of the siblings allegedly began to shoot about 20 rounds at the police cruiser. The cop car was disabled and the gang escaped.

Later that day, the outlaws entered a bank in Valdosta, Ga., 15 miles north of the border with Florida, dressed in black and carrying two weapons, including what looked like an AK-47 assault rifle. They fired shots at the ceiling and demanded cash before fleeing, according to the FBI.

The siblings' mother, Barbara Bell, pleaded for her children to turn themselves in during an interview with a local news station. 

"You've made some bad mistakes, but so far no one has been physically harmed," Bell told WFTS-TV. "The only safe thing, the only right thing, the only good thing -- possible thing to do -- is for you to turn yourselves in." 

"I love you," she said. 

Lee Grace has been arrested several times for battery. Earlier this year, she was charged in a hit-and-run accident, just 10 days after being arrested for DUI and battery of a law enforcement officer, according to the St. Petersburg Times. On her photo-sharing Flickr account, she describes herself as a proud "redneck," who loves "to farm and shoot guys and wreck cars" and says she likes "milk and German engineering and causing mayhem with my siblings."

Ryan Dougherty -- whose prior arrests included battery, burglary, destroying evidence and possession of methamphetamine -- recently was sentenced to 10 years probation for sexual battery after sending explicit text messages to an 11-year-old girl, according to the St. Petersburg Times. He is believed to have cut off an ankle monitor just before last week's crime spree began.

Their brother, Dylan Dougherty Stanley, with the shortest criminal record, was once arrested for marijuana possession.